Harris was born on 14 August 1810 to William Harris, 2nd Baron Harris and his wife Eliza Selina Anne who owned Waterstown House at Glasson, Co. Westmeath, Ireland, and Belmont House, Faversham, England. He was the grandson of George Harris, 1st Baron Harris, who had commanded the army of the British East India Company in the Fourth Mysore War. Harris had his early education at Eton College and under the private tutorship of Rev. John Shaw before joining Merton College, Oxford in 1829. Harris completed his matriculation from Merton College and graduated in arts from Christ Church, Oxford in 1832. He succeeded his father in June 1845 to the barony and the family seat of Belmont House. He also became joint patron of Athlone Yacht Club in 1845 with Lord Castlemaine and Hon. L. H. King-Harman following the death of his father. Harris was beset will ill-health and remained bed-ridden for some time in the city ofPau in France where he worked for a time for the Church of England.
Governor of Trinidad
In 1846, Harris was appointed Governor of Trinidad, a role he kept until 1854. In 1850 he married Sarah, daughter of Port of Spain archdeacon George Cummins. During his tenure, Harris revamped the prevailing education system thereby laying down the foundation for the present-day system of education prevailing in Trinidad. Harris also mooted the idea of importing indentured labourers from India to replace the plantation slaves who had been freed following the abolition of slavery. Harris is considered to be one of Trinidad's best ever administrators though he had also been criticized for favouring his own men in appointments.
Governor of Madras
Soon after taking over as Governor of Madras, Harris found grave deficiencies in the police system in the Presidency and reorganised the force introducing reforms that would eventually give rise to the Indian police as it exists today. On 1 July 1856, Harris flagged off the first regular passenger train service in the province between the city of Madras and the town of Arcot. The University of Madras was established in 1857 when Harris was the governor. In September 1854, Harris headed the Torture Commission appointed to investigate the allegations of torture inflicted on Indian peasants by revenue officials. Throughout his tenure, Harris was critical of the attitude of the Anglo-Indian press in Madras and tried to regulate the freedom of the press. He criticized them as: When the Indian Rebellion of 1857 broke out, the province of Madras remained loyal to the British Crown. As a result, Harris lent the whole Madras Army to the Government of India for quelling the rebellion. The Madras Army participated in the relief of Cawnpore in which Lieutenant-ColonelJames George Smith Neill of the Madras Fusiliers indulged in indiscriminate massacre of Indians and was eventually killed. However, there is also evidence that suggests that one of the 52 regiments of the Madras Army refused to volunteer for service during the mutiny. Harris continued even after the transfer of sovereignty over India from the British East India Company to the British crown in 1858, eventually resigning as governor in 1859.
Lord Harris died in November 1872, aged 62. In 1850 he had married Sarah, daughter of the Venerable George Cummons, Archdeacon of Trinidad. She died only three years later. Lord Harris was succeeded in the barony by his son Robert Harris, 4th Baron Harris, who became a successful cricketer and Conservative politician.